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  • Küçük Resim Yok
    Öğe
    Hydrogen evolution at polarised liquid/liquid interfaces catalyzed by molybdenum disulfide
    (ROYAL SOC CHEMISTRY, 2011) Hatay, Imren; Ge, Pei Yu; Vrubel, Heron; Hu, Xile; Girault, Hubert H.
    Molybdenum disulfide microparticles in suspension in an aqueous acidic solution adsorb at the interface with an organic electrolyte solution containing the reducing agent, decamethylferrocene, to catalyse hydrogen evolution. This catalytic process has been investigated by voltammetry at the water/1,2-dichloroethane interface and by biphasic reactions monitored by gas chromatography and UV-visible spectroscopy.
  • Küçük Resim
    Öğe
    Oxygen and Proton Reduction by Decamethylferrocene in Non-Aqueous Acidic Media
    (Royal Soc Chemistry, 2010) Su, Bin; Hatay, İmren; Ge, Pei Yu; Mendez, Manuel; Corminboeuf, Clemence; Samec, Zdenek; Ersöz, Mustafa; Girault, Hubert H.
    Experimental studies and density functional theory (DFT) computations suggest that oxygen and proton reduction by decamethylferrocene (DMFc) in 1,2-dichloroethane involves protonated DMFc, DMFcH(+), as an active intermediate species, producing hydrogen peroxide and hydrogen in aerobic and anaerobic conditions, respectively.